As adjectives the difference between unpolled and untolled
is that unpolled is not polled (included in a vote) while untolled is on which no toll is charged.
unpolled
English
Adjective
(-)
Not polled (included in a vote).
untolled
English
Adjective
(-)
On which no toll is charged.
(rare, poetic) Not having been tolled; unrung.